High-Energy SiO-Sulfur Battery with Preloaded Li3N in a Cathode as a Lithiation Reagent
The practical use of lithium-sulfur batteries faces the "shuttle effect" and lithium dendrite growth. Employing SiO instead of Li metal can fundamentally solve the above problems. Nevertheless, selecting a convenient prelithiation method is essential for normal operation of the battery system. Hence, this work proposed a novel SiO-sulfur battery with preloaded Li3N in a cathode as a prelithiation reagent, which can thoroughly solve the dendrite problem and the side reaction with polysulfides of lithium anode. The SKB-Li3N vs SiO full cell can obtain a high specific capacity of 790 mAh g-1 after the activation process and be maintained at 478 mAh g-1 after 100 cycles. Our design will provide a new prelithiation strategy for a high-specific-energy SiO-sulfur battery system.
| Medienart: |
E-Artikel |
|---|
| Erscheinungsjahr: |
2024 |
|---|---|
| Erschienen: |
2024 |
| Enthalten in: |
Zur Gesamtaufnahme - volume:40 |
|---|---|
| Enthalten in: |
Langmuir : the ACS journal of surfaces and colloids - 40(2024), 16 vom: 23. Apr., Seite 8678-8684 |
| Sprache: |
Englisch |
|---|
| Beteiligte Personen: |
Wang, Peng-Fei [VerfasserIn] |
|---|
| Links: |
|---|
| Themen: |
|---|
| Anmerkungen: |
Date Revised 23.04.2024 published: Print-Electronic Citation Status PubMed-not-MEDLINE |
|---|
| doi: |
10.1021/acs.langmuir.4c00484 |
|---|
| funding: |
|
|---|---|
| Förderinstitution / Projekttitel: |
|
| PPN (Katalog-ID): |
NLM370958926 |
|---|
| LEADER | 01000caa a22002652 4500 | ||
|---|---|---|---|
| 001 | NLM370958926 | ||
| 003 | DE-627 | ||
| 005 | 20240424232205.0 | ||
| 007 | cr uuu---uuuuu | ||
| 008 | 240412s2024 xx |||||o 00| ||eng c | ||
| 024 | 7 | |a 10.1021/acs.langmuir.4c00484 |2 doi | |
| 028 | 5 | 2 | |a pubmed24n1385.xml |
| 035 | |a (DE-627)NLM370958926 | ||
| 035 | |a (NLM)38606578 | ||
| 040 | |a DE-627 |b ger |c DE-627 |e rakwb | ||
| 041 | |a eng | ||
| 100 | 1 | |a Wang, Peng-Fei |e verfasserin |4 aut | |
| 245 | 1 | 0 | |a High-Energy SiO-Sulfur Battery with Preloaded Li3N in a Cathode as a Lithiation Reagent |
| 264 | 1 | |c 2024 | |
| 336 | |a Text |b txt |2 rdacontent | ||
| 337 | |a ƒaComputermedien |b c |2 rdamedia | ||
| 338 | |a ƒa Online-Ressource |b cr |2 rdacarrier | ||
| 500 | |a Date Revised 23.04.2024 | ||
| 500 | |a published: Print-Electronic | ||
| 500 | |a Citation Status PubMed-not-MEDLINE | ||
| 520 | |a The practical use of lithium-sulfur batteries faces the "shuttle effect" and lithium dendrite growth. Employing SiO instead of Li metal can fundamentally solve the above problems. Nevertheless, selecting a convenient prelithiation method is essential for normal operation of the battery system. Hence, this work proposed a novel SiO-sulfur battery with preloaded Li3N in a cathode as a prelithiation reagent, which can thoroughly solve the dendrite problem and the side reaction with polysulfides of lithium anode. The SKB-Li3N vs SiO full cell can obtain a high specific capacity of 790 mAh g-1 after the activation process and be maintained at 478 mAh g-1 after 100 cycles. Our design will provide a new prelithiation strategy for a high-specific-energy SiO-sulfur battery system | ||
| 650 | 4 | |a Journal Article | |
| 700 | 1 | |a Wang, Jian-Cang |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Nan |e verfasserin |4 aut | |
| 700 | 1 | |a Tian, Shu-Hui |e verfasserin |4 aut | |
| 700 | 1 | |a Yi, Ting-Feng |e verfasserin |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Langmuir : the ACS journal of surfaces and colloids |d 1992 |g 40(2024), 16 vom: 23. Apr., Seite 8678-8684 |w (DE-627)NLM098181009 |x 1520-5827 |7 nnns |
| 773 | 1 | 8 | |g volume:40 |g year:2024 |g number:16 |g day:23 |g month:04 |g pages:8678-8684 |
| 856 | 4 | 0 | |u http://dx.doi.org/10.1021/acs.langmuir.4c00484 |3 Volltext |
| 912 | |a GBV_USEFLAG_A | ||
| 912 | |a GBV_NLM | ||
| 951 | |a AR | ||
| 952 | |d 40 |j 2024 |e 16 |b 23 |c 04 |h 8678-8684 | ||