Photocatalytic oxidation of formaldehyde under visible light using BiVO4-TiO2 synthesized via ultrasonic blending
© 2024. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature..
Formaldehyde (HCHO) is one of the primary indoor air pollutants, and efficiently eliminating it, especially at low concentrations, remains challenging. In this study, BiVO4-TiO2 catalyst was developed using ultrasonic blending technology for the photocatalytic oxidation of low-level indoor HCHO. The crystal structure, surface morphology, element distribution, and active oxidation species of the catalyst were examined using XRD, SEM, TEM, UV-Vis, EDS, and ESR techniques. Our results demonstrated that the BiVO4-TiO2 catalyst, prepared by ultrasonic blending, exhibited good oxidation performance and stability. The HCHO concentration reduced from 1.050 to 0.030 mg/m3 within 48 h, achieving a removal rate of 97.1%. The synergy between BiVO4 and TiO2 enhanced the efficiency of separating photogenerated carriers and minimized the likelihood of recombination between photogenerated electrons and holes. Additionally, this synergy significantly enhanced the presence of hydroxyl radicals (·OH) on the catalyst, resulting in an oxidation performance superior to that of either BiVO4 or TiO2. Our research offers valuable insights for the development of new photocatalysts to address HCHO pollution.
Medienart: |
E-Artikel |
---|
Erscheinungsjahr: |
2024 |
---|---|
Erschienen: |
2024 |
Enthalten in: |
Zur Gesamtaufnahme - year:2024 |
---|---|
Enthalten in: |
Environmental science and pollution research international - (2024) vom: 10. Apr. |
Sprache: |
Englisch |
---|
Beteiligte Personen: |
Yang, Jingyi [VerfasserIn] |
---|
Links: |
---|
Themen: |
Bismuth vanadate |
---|
Anmerkungen: |
Date Revised 10.04.2024 published: Print-Electronic Citation Status Publisher |
---|
doi: |
10.1007/s11356-024-33192-2 |
---|
funding: |
|
---|---|
Förderinstitution / Projekttitel: |
|
PPN (Katalog-ID): |
NLM370874889 |
---|
LEADER | 01000naa a22002652 4500 | ||
---|---|---|---|
001 | NLM370874889 | ||
003 | DE-627 | ||
005 | 20240410233653.0 | ||
007 | cr uuu---uuuuu | ||
008 | 240410s2024 xx |||||o 00| ||eng c | ||
024 | 7 | |a 10.1007/s11356-024-33192-2 |2 doi | |
028 | 5 | 2 | |a pubmed24n1371.xml |
035 | |a (DE-627)NLM370874889 | ||
035 | |a (NLM)38598155 | ||
040 | |a DE-627 |b ger |c DE-627 |e rakwb | ||
041 | |a eng | ||
100 | 1 | |a Yang, Jingyi |e verfasserin |4 aut | |
245 | 1 | 0 | |a Photocatalytic oxidation of formaldehyde under visible light using BiVO4-TiO2 synthesized via ultrasonic blending |
264 | 1 | |c 2024 | |
336 | |a Text |b txt |2 rdacontent | ||
337 | |a ƒaComputermedien |b c |2 rdamedia | ||
338 | |a ƒa Online-Ressource |b cr |2 rdacarrier | ||
500 | |a Date Revised 10.04.2024 | ||
500 | |a published: Print-Electronic | ||
500 | |a Citation Status Publisher | ||
520 | |a © 2024. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature. | ||
520 | |a Formaldehyde (HCHO) is one of the primary indoor air pollutants, and efficiently eliminating it, especially at low concentrations, remains challenging. In this study, BiVO4-TiO2 catalyst was developed using ultrasonic blending technology for the photocatalytic oxidation of low-level indoor HCHO. The crystal structure, surface morphology, element distribution, and active oxidation species of the catalyst were examined using XRD, SEM, TEM, UV-Vis, EDS, and ESR techniques. Our results demonstrated that the BiVO4-TiO2 catalyst, prepared by ultrasonic blending, exhibited good oxidation performance and stability. The HCHO concentration reduced from 1.050 to 0.030 mg/m3 within 48 h, achieving a removal rate of 97.1%. The synergy between BiVO4 and TiO2 enhanced the efficiency of separating photogenerated carriers and minimized the likelihood of recombination between photogenerated electrons and holes. Additionally, this synergy significantly enhanced the presence of hydroxyl radicals (·OH) on the catalyst, resulting in an oxidation performance superior to that of either BiVO4 or TiO2. Our research offers valuable insights for the development of new photocatalysts to address HCHO pollution | ||
650 | 4 | |a Journal Article | |
650 | 4 | |a Bismuth vanadate | |
650 | 4 | |a Formaldehyde | |
650 | 4 | |a Heterojunction | |
650 | 4 | |a Photocatalytic oxidation | |
650 | 4 | |a Titanium dioxide | |
700 | 1 | |a Huang, Qiong |e verfasserin |4 aut | |
700 | 1 | |a Sun, Yueyin |e verfasserin |4 aut | |
700 | 1 | |a An, Guofang |e verfasserin |4 aut | |
700 | 1 | |a Li, Xin |e verfasserin |4 aut | |
700 | 1 | |a Mao, Junjie |e verfasserin |4 aut | |
700 | 1 | |a Wei, Chen |e verfasserin |4 aut | |
700 | 1 | |a Yang, Bo |e verfasserin |4 aut | |
700 | 1 | |a Li, Dawei |e verfasserin |4 aut | |
700 | 1 | |a Tao, Tao |e verfasserin |4 aut | |
700 | 1 | |a Yang, Hong |e verfasserin |4 aut | |
773 | 0 | 8 | |i Enthalten in |t Environmental science and pollution research international |d 1994 |g (2024) vom: 10. Apr. |w (DE-627)NLM093849869 |x 1614-7499 |7 nnns |
773 | 1 | 8 | |g year:2024 |g day:10 |g month:04 |
856 | 4 | 0 | |u http://dx.doi.org/10.1007/s11356-024-33192-2 |3 Volltext |
912 | |a GBV_USEFLAG_A | ||
912 | |a GBV_NLM | ||
951 | |a AR | ||
952 | |j 2024 |b 10 |c 04 |