Total Synthesis of Quebrachamine and Kopsiyunnanine D
The total syntheses of (±)-quebrachamine and (±)-kopsiyunnanine D are reported. Key transformations include an intermolecular Horner-Wadsworth-Emmons olefination to merge the two fragments convergently and an intramolecular Mitsunobu reaction to introduce the synthetically challenging nine-membered azonane ring efficiently.
| Medienart: |
E-Artikel |
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| Erscheinungsjahr: |
2024 |
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| Erschienen: |
2024 |
| Enthalten in: |
Zur Gesamtaufnahme - volume:89 |
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| Enthalten in: |
The Journal of organic chemistry - 89(2024), 8 vom: 19. Apr., Seite 5905-5910 |
| Sprache: |
Englisch |
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| Beteiligte Personen: |
Liu, Hui [VerfasserIn] |
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| Links: |
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| Themen: |
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| Anmerkungen: |
Date Revised 19.04.2024 published: Print-Electronic Citation Status PubMed-not-MEDLINE |
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| doi: |
10.1021/acs.joc.4c00363 |
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| funding: |
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| Förderinstitution / Projekttitel: |
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| PPN (Katalog-ID): |
NLM370685857 |
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| 520 | |a The total syntheses of (±)-quebrachamine and (±)-kopsiyunnanine D are reported. Key transformations include an intermolecular Horner-Wadsworth-Emmons olefination to merge the two fragments convergently and an intramolecular Mitsunobu reaction to introduce the synthetically challenging nine-membered azonane ring efficiently | ||
| 650 | 4 | |a Journal Article | |
| 700 | 1 | |a Yuan, Wei |e verfasserin |4 aut | |
| 700 | 1 | |a Ran, Meng-Yan |e verfasserin |4 aut | |
| 700 | 1 | |a Wei, Gang |e verfasserin |4 aut | |
| 700 | 1 | |a Zhao, Yi |e verfasserin |4 aut | |
| 700 | 1 | |a Liao, Zhi-Qiang |e verfasserin |4 aut | |
| 700 | 1 | |a Liang, Hong |e verfasserin |4 aut | |
| 700 | 1 | |a Chen, Zhen-Feng |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Fang-Xin |e verfasserin |4 aut | |
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