Highly elastic, fatigue-resistant, antibacterial, conductive, and nanocellulose-enhanced hydrogels with selenium nanoparticles loading as strain sensors

Copyright © 2024 Elsevier Ltd. All rights reserved..

The fabrication of highly elastic, fatigue-resistant and conductive hydrogels with antibacterial properties is highly desirable in the field of wearable devices. However, it remains challenging to simultaneously realize the above properties within one hydrogel without compromising excellent sensing ability. Herein, we fabricated a highly elastic, fatigue-resistant, conductive, antibacterial and cellulose nanocrystal (CNC) enhanced hydrogel as a sensitive strain sensor by the synergistic effect of biosynthesized selenium nanoparticles (BioSeNPs), MXene and nanocellulose. The structure and potential mechanism to generate biologically synthesized SeNPs (BioSeNPs) were systematically investigated, and the role of protease A (PrA) in enhancing the adsorption between proteins and SeNPs was demonstrated. Additionally, owing to the incorporation of BioSeNPs, CNC and MXene, the synthesized hydrogels showed high elasticity, excellent fatigue resistance and antibacterial properties. More importantly, the sensitivity of hydrogels determined by the gauge factor was as high as 6.24 when a high strain was applied (400-700 %). This study provides a new horizon to synthesize high-performance antibacterial and conductive hydrogels for soft electronics applications.

Medienart:

E-Artikel

Erscheinungsjahr:

2024

Erschienen:

2024

Enthalten in:

Zur Gesamtaufnahme - volume:334

Enthalten in:

Carbohydrate polymers - 334(2024) vom: 15. Apr., Seite 122068

Sprache:

Englisch

Beteiligte Personen:

Nie, Xinling [VerfasserIn]
Xie, Yitong [VerfasserIn]
Ding, Xiaofeng [VerfasserIn]
Dai, Lili [VerfasserIn]
Gao, Feng [VerfasserIn]
Song, Wancheng [VerfasserIn]
Li, Xun [VerfasserIn]
Liu, Pei [VerfasserIn]
Tan, Zhongbiao [VerfasserIn]
Shi, Hao [VerfasserIn]
Lai, Chenhuan [VerfasserIn]
Zhang, Daihui [VerfasserIn]
Lai, Yongxian [VerfasserIn]

Links:

Volltext

Themen:

9004-34-6
Anti-Bacterial Agents
Cellulose
H6241UJ22B
Hydrogel
Hydrogels
Journal Article
MXene
Nanocellulose
Nitrites
Selenium
Selenium nanoparticles
Transition Elements
Wearable device

Anmerkungen:

Date Completed 01.04.2024

Date Revised 01.04.2024

published: Print-Electronic

Citation Status MEDLINE

doi:

10.1016/j.carbpol.2024.122068

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM370427262