Monolayer V_{2}MX_{4} : A New Family of Quantum Anomalous Hall Insulators

We theoretically propose that the van der Waals layered ternary transition metal chalcogenide V_{2}MX_{4} (M=W, Mo; X=S, Se) is a new family of quantum anomalous Hall insulators with sizable bulk gap and Chern number C=-1. The large topological gap originates from the deep band inversion between spin-up bands contributed by d_{xz}, d_{yz} orbitals of V and spin-down band from d_{z^{2}} orbital of M at the Fermi level. Remarkably, the Curie temperature of monolayer V_{2}MX_{4} is predicted to be much higher than that of monolayer MnBi_{2}Te_{4}. Furthermore, the thickness dependence of the Chern number for few multilayers shows interesting oscillating behavior. The general physics from the d orbitals here applies to a large class of ternary transition metal chalcogenide such as Ti_{2}WX_{4} with the space group P-42m. These interesting predictions, if realized experimentally, could greatly promote the research and application of topological quantum physics.

Medienart:

E-Artikel

Erscheinungsjahr:

2024

Erschienen:

2024

Enthalten in:

Zur Gesamtaufnahme - volume:132

Enthalten in:

Physical review letters - 132(2024), 10 vom: 08. März, Seite 106602

Sprache:

Englisch

Beteiligte Personen:

Jiang, Yadong [VerfasserIn]
Wang, Huan [VerfasserIn]
Bao, Kejie [VerfasserIn]
Liu, Zhaochen [VerfasserIn]
Wang, Jing [VerfasserIn]

Links:

Volltext

Themen:

Journal Article

Anmerkungen:

Date Revised 22.03.2024

published: Print

Citation Status PubMed-not-MEDLINE

doi:

10.1103/PhysRevLett.132.106602

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM370078772