Spectral and temporal atomic coherence interaction in Eu3+ : NaYF4 and Eu3+ : BiPO4

We investigate the spectral and temporal atomic coherence interaction based on out-of-phase fluorescence (FL) and spontaneous parametric four-wave mixing (SFWM) from the hexagonal phase of Eu3+ : NaYF4 and different phases of Eu3+ : BiPO4. Spectral and temporal interactions are interrelated and reduced by about 2 times due to two-photon nested dressing in contrast to the sum of each laser excitation. As the lifetime of photons increases, off-resonance profile cross-interaction decreases because cross-interaction reverses the signal at the near time gate position and keeps it consistent at the far time gate position. Moreover, the thermal phonon dressing at 300 K exhibits 6 times more eminent and obvious temporal interaction than that at 77 K. In a different phase of Eu3+ : BiPO4, there are three dark dips having stronger self-interaction; however, Eu3+ : NaYF4 has two dark dips as Eu3+ : BiPO4 has two phonon dressing. Further, the pure hexagonal phase of Eu3+ : BiPO4 demonstrates the strongest cross-interaction and longest coherent time under the dressing effect due to the smallest dressing phonon detuning and off-resonance profile cross-interaction at PMT2 because the angle quantization is the strongest. Such results can be used for designing novel quantum devices and have potential applications in quantum memory devices.

Medienart:

E-Artikel

Erscheinungsjahr:

2024

Erschienen:

2024

Enthalten in:

Zur Gesamtaufnahme - volume:26

Enthalten in:

Physical chemistry chemical physics : PCCP - 26(2024), 3 vom: 17. Jan., Seite 2486-2496

Sprache:

Englisch

Beteiligte Personen:

Feng, Zhou [VerfasserIn]
Imran, Muhammad [VerfasserIn]
Nadeem, Faisal [VerfasserIn]
Fan, Huanrong [VerfasserIn]
Yan, Jin [VerfasserIn]
Ahmed, Irfan [VerfasserIn]
Lau, Condon [VerfasserIn]
Zhang, Yanpeng [VerfasserIn]

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Date Revised 06.02.2024

published: Electronic

Citation Status PubMed-not-MEDLINE

doi:

10.1039/d3cp00775h

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM366612654