Unique and outstanding catalytic behavior of a novel MOFCOF composite as an emerging and powerful catalyst in the preparation of 2,3-dihydroquinazolin-4(1H)-one derivatives
This journal is © The Royal Society of Chemistry..
The creation of an emerging porous structure using the hybridization of UiO-66-NH2-MOF, a zirconium-based metal-organic framework (MOF), with a covalent organic framework (COF) based on terephthaldehyde and melamine (UiO-66-NH2-MOFCOF), was assessed using SEM, XRD, EDX/mapping, FT-IR, BET, and TGA analyses. Using the obtained composite as a potential recoverable heterogeneous nanocatalyst, different aldehydes were condensed with isatoic anhydride and anilines or ammonium acetate under solvent-free conditions to create derivatives of 2,3-dihydroquinazolin-4(1H)-one. Examining the catalytic capabilities of the designed UiO-66-NH2-MOF@COF to efficiently produce 2,3-dihydroquinazolin-4(1H)-ones was a standout activity. Low catalyst loading, simple set-up, outstanding yields, and catalyst recoverability are all benefits of this research.
| Medienart: |
E-Artikel |
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| Erscheinungsjahr: |
2023 |
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| Erschienen: |
2023 |
| Enthalten in: |
Zur Gesamtaufnahme - volume:5 |
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| Enthalten in: |
Nanoscale advances - 5(2023), 24 vom: 05. Dez., Seite 7031-7041 |
| Sprache: |
Englisch |
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| Beteiligte Personen: |
Ghasemzadeh, Mohammad Ali [VerfasserIn] |
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| Links: |
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| Anmerkungen: |
Date Revised 08.12.2023 published: Electronic-eCollection Citation Status PubMed-not-MEDLINE |
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| doi: |
10.1039/d3na00805c |
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| funding: |
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| Förderinstitution / Projekttitel: |
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| 245 | 1 | 7 | |a Unique and outstanding catalytic behavior of a novel MOFCOF composite as an emerging and powerful catalyst in the preparation of 2,3-dihydroquinazolin-4(1H)-one derivatives |
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| 520 | |a The creation of an emerging porous structure using the hybridization of UiO-66-NH2-MOF, a zirconium-based metal-organic framework (MOF), with a covalent organic framework (COF) based on terephthaldehyde and melamine (UiO-66-NH2-MOFCOF), was assessed using SEM, XRD, EDX/mapping, FT-IR, BET, and TGA analyses. Using the obtained composite as a potential recoverable heterogeneous nanocatalyst, different aldehydes were condensed with isatoic anhydride and anilines or ammonium acetate under solvent-free conditions to create derivatives of 2,3-dihydroquinazolin-4(1H)-one. Examining the catalytic capabilities of the designed UiO-66-NH2-MOF@COF to efficiently produce 2,3-dihydroquinazolin-4(1H)-ones was a standout activity. Low catalyst loading, simple set-up, outstanding yields, and catalyst recoverability are all benefits of this research | ||
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