Advances in Inorganic Solid-State Electrolyte/Li Interface

© 2023 Wiley-VCH GmbH..

The increasing demand for high-energy-density and high-safety energy storage devices has sparked a growing interest in all-solid-state lithium metal batteries (ASSLMBs). A high-quality inorganic solid-state electrolyte (ISE) is a fundamental requirement for ASSLMBs, and an effective ISE/Li interface is a key factor in attaining high-performance ASSLMBs. In this Concept, we initially summarize the challenges encountered by ISE/Li interfaces and delineate four commonly employed strategies for modifying the ISE/Li interface. Then, we explore the merits and drawbacks of coatings utilized as ISE/Li interfacial phases. We also delve into the commonly employed thermal bonding and innovative cold bonding methods utilized for in situ interface preparation. Lastly, we spotlight future directions for enhancing the functionality of ISE/Li interfaces and achieving high-performance ASSLMBs.

Medienart:

E-Artikel

Erscheinungsjahr:

2024

Erschienen:

2024

Enthalten in:

Zur Gesamtaufnahme - volume:30

Enthalten in:

Chemistry (Weinheim an der Bergstrasse, Germany) - 30(2024), 5 vom: 22. Jan., Seite e202303454

Sprache:

Englisch

Beteiligte Personen:

Chen, Yi [VerfasserIn]
Qian, Ji [VerfasserIn]
Li, Li [VerfasserIn]
Wu, Feng [VerfasserIn]
Chen, Renjie [VerfasserIn]

Links:

Volltext

Themen:

All-solid-state lithium metal batteries
Coatings
Cold bonding
Inorganic solid-state electrolyte
Interfacial modification
Journal Article

Anmerkungen:

Date Revised 23.01.2024

published: Print-Electronic

Citation Status PubMed-not-MEDLINE

doi:

10.1002/chem.202303454

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM364541482