Unexpectedly rapid aerosol formation in the Hunga Tonga plume

The Hunga Tonga-Hunga Ha'apai (HT-HH) volcanic eruptions on January 13 and 15, 2022, produced a plume with the highest signal in stratospheric aerosol optical depth observed since the eruption of Mt. Pinatubo in 1991. Suites of balloon-borne instruments on a series of launches from Réunion Island intercepted the HT-HH plume between 7 and 10 d of the eruptions, yielding observations of the aerosol number and size distribution and sulfur dioxide (SO2) and water vapor (H2O) concentrations. The measurements reveal an unexpected abundance of large particles in the plume, constrain the total sulfur injected to approximately 0.2 Tg, provide information on the altitude of the injection, and indicate that the formation of sulfuric acid aerosol was complete within 3 wk. Large H2O enhancements contributed as much as ~30% to ambient aerosol surface area and likely accelerated SO2 oxidation and aerosol formation rates in the plume to approximately three times faster than under normal stratospheric conditions.

Medienart:

E-Artikel

Erscheinungsjahr:

2023

Erschienen:

2023

Enthalten in:

Zur Gesamtaufnahme - volume:120

Enthalten in:

Proceedings of the National Academy of Sciences of the United States of America - 120(2023), 46 vom: 14. Nov., Seite e2219547120

Sprache:

Englisch

Beteiligte Personen:

Asher, Elizabeth [VerfasserIn]
Todt, Michael [VerfasserIn]
Rosenlof, Karen [VerfasserIn]
Thornberry, Troy [VerfasserIn]
Gao, Ru-Shan [VerfasserIn]
Taha, Ghassan [VerfasserIn]
Walter, Paul [VerfasserIn]
Alvarez, Sergio [VerfasserIn]
Flynn, James [VerfasserIn]
Davis, Sean M [VerfasserIn]
Evan, Stephanie [VerfasserIn]
Brioude, Jerome [VerfasserIn]
Metzger, Jean-Marc [VerfasserIn]
Hurst, Dale F [VerfasserIn]
Hall, Emrys [VerfasserIn]
Xiong, Kensy [VerfasserIn]

Links:

Volltext

Themen:

Hunga Tonga eruption
Journal Article
Rapid aerosol formation
SO2
Stratospheric aerosol
Volcanic plume

Anmerkungen:

Date Revised 19.11.2023

published: Print-Electronic

Citation Status PubMed-not-MEDLINE

doi:

10.1073/pnas.2219547120

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM363952284