Atomically thin PdSeO3 nanosheets : a promising 2D photocatalyst produced by quaternary ammonium intercalation and exfoliation

In 2018, the two-dimensional (2D) PdSeO3 monolayer was predicted to be a highly promising photocatalyst for direct overall water splitting in the light of density functional theory (DFT) computations. Herein, we present the first report on the synthesis of 2D PdSeO3 nanosheets by using the quaternary ammonium intercalation-assisted electrochemical exfoliation method. The resulting atomically thin PdSeO3 nanosheets possess a moderate band gap with suitable band edge alignments for water splitting, and display excellent activity and stability in photocatalytic H2 evolution.

Medienart:

E-Artikel

Erscheinungsjahr:

2020

Erschienen:

2020

Enthalten in:

Zur Gesamtaufnahme - volume:56

Enthalten in:

Chemical communications (Cambridge, England) - 56(2020), 41 vom: 21. Mai, Seite 5504-5507

Sprache:

Englisch

Beteiligte Personen:

Zhang, Xiuming [VerfasserIn]
Liu, Jia [VerfasserIn]
Zhang, Erhuang [VerfasserIn]
Pan, Rongrong [VerfasserIn]
Li, Yuemei [VerfasserIn]
Wan, Xiaodong [VerfasserIn]
Wang, Hongzhi [VerfasserIn]
Zhang, Jiatao [VerfasserIn]

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Date Revised 21.05.2020

published: Print-Electronic

Citation Status PubMed-not-MEDLINE

doi:

10.1039/d0cc01642j

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM308816927