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1 |
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|a Li, Hebin
|e verfasserin
|4 aut
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| 245 |
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|a Optical multidimensional coherent spectroscopy
|c Hebin Li, Bachana Lomsadze, Galan Moody, Chris Smallwood, Steven Cundiff
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| 264 |
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|a Oxford
|a New York, NY
|b Oxford University Press
|c 2023
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| 300 |
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|a 1 Online-Ressource
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| 336 |
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|a Text
|b txt
|2 rdacontent
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|a Includes bibliographical references and index
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|a Cover -- titlepage -- copyright -- dedication -- preface -- Acknowledgements -- Table of symbols -- Table of acronyms -- contents -- Basics of ultrafast spectroscopy -- Basics of spectroscopy: linear versus nonlinear -- Ultrashort pulses -- Ultrafast nonlinear/coherent spectroscopy -- The density matrix -- Bloch sphere representation of quantum states -- Introduction to multidimensional coherent spectroscopy -- Concepts of multidimensional coherent spectroscopy -- Coherent spectroscopy -- Multidimensional coherent spectroscopy -- Spectrum classification
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| 505 |
8 |
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|a Density matrix formalism and double-sided Feynman diagrams -- Interpreting MDCS in the perturbative limit -- Double-sided Feynman diagrams -- Measured observables -- Putting it all together -- Case study: Two-level system -- Phase matching -- Two-dimensional infrared (2D IR) spectroscopy -- Interpretation of multidimensional coherent spectra -- Isolated two-level system -- Inhomogeneously broadened ensemble of two-level systems -- Gaussian inhomogeneity, constant homogeneous linewidth -- Large inhomogeneity -- Coherent coupling signatures -- Incoherent coupling signatures
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| 505 |
8 |
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|a Doubly excited states and many-body interactions -- Double-quantum spectra -- Zero-quantum spectra -- Three-dimensional coherent spectroscopy -- Nonrephasing pathways and purely absorptive spectra -- Finite-pulse effects -- Mathematical formulations -- Example spectra -- Further applications -- Experimental implementations -- Experimental requirements and considerations -- Precision and stability of time delays -- Isolation of the signal -- Detection of the signal -- Overview of experimental approaches -- Actively stabilized box geometry -- Phase modulated collinear geometry
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| 505 |
8 |
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|a Comparison of different approaches -- Data analysis -- Multidimensional coherent spectroscopy of atomic ensembles -- Single- and zero-quantum 2D spectra of atomic vapors -- MDCS in optically thick samples -- Probing many-body interactions with double-quantum 2D spectroscopy -- Probing many-body correlations with multi-quantum 2D spectroscopy -- Frequency comb-based multidimensional coherent spectroscopy -- Introduction to frequency combs and dual-comb spectroscopy -- Frequency comb-based four-wave-mixing spectroscopy -- Frequency comb-based single-quantum 2D spectroscopy
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| 505 |
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|a Frequency comb-based double-quantum 2D spectroscopy -- Tri-comb spectroscopy -- Two-dimensional spectroscopy of semiconductor quantum wells -- Introduction to semiconductor optics -- Many-body signatures in one-quantum 2D spectra -- Many-body signatures in double- and multi-quantum 2D spectra -- Two-dimensional spectroscopy of coupled quantum wells -- Quantum well exciton-polaritons in microcavities -- Three-dimensional coherent spectroscopy -- Fifth-order 3D infrared spectroscopy -- Fifth-order 3D electronic spectroscopy -- Third-order 3D electronic spectroscopy
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| 520 |
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|a Aimed at post-doctoral scientists, researchers, and graduate students in physics, this book provides an introduction to optical multidimensional coherent spectroscopy, a relatively new method of studying materials based on using ultrashort light pulses to perform spectroscopy
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| 650 |
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|a Optical spectroscopy
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| 650 |
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4 |
|a Optical spectroscopy
|0 (OCoLC)fst01739874
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| 650 |
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|a Chemistry
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| 650 |
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4 |
|a Science
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4 |
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