A novel 3D coordination polymer constructed by dual-ligand for highly sensitive detection of purine metabolite uric acid
Copyright © 2021. Published by Elsevier B.V..
Uric acid (UA), as the final product of purine metabolism, exists in urine and serum, which plays an important role in human metabolism, immunity and other functions. The sensitive, efficient, and rapid detection of UA has far-reaching significance in clinical diagnosis and disease prevention. Herein, a novel coordination polymer constructed by dual-ligand was successfully prepared, which exhibited excellent thermal and water stability. The polymer was interlaced by coordination bonds and hydrogen bonds to form an infinitely extended three-dimensional framework, which showed a rare and novel topological structure. The complex selectively recognized UA through significant fluorescence quenching response in the presence of various interferences. The excellent detection sensitivity (the limited detection of 1.2 μM), outstanding anti-interference ability and remarkable recyclability marked the complex to be a promising sensor material towards UA. In addition, the detection mechanism of UA by the complex was investigated in detail by combining density functional theory (DFT) and a variety of other analytical methods.
| Medienart: |
E-Artikel |
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| Erscheinungsjahr: |
2021 |
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| Erschienen: |
2021 |
| Enthalten in: |
Zur Gesamtaufnahme - volume:262 |
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| Enthalten in: |
Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy - 262(2021) vom: 05. Dez., Seite 120065 |
| Sprache: |
Englisch |
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| Beteiligte Personen: |
Zhao, Xiao-Yang [VerfasserIn] |
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| Links: |
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| Themen: |
268B43MJ25 |
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| Anmerkungen: |
Date Completed 27.07.2021 Date Revised 27.07.2021 published: Print-Electronic Citation Status MEDLINE |
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| doi: |
10.1016/j.saa.2021.120065 |
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| funding: |
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| Förderinstitution / Projekttitel: |
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| PPN (Katalog-ID): |
NLM327448393 |
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| 100 | 1 | |a Zhao, Xiao-Yang |e verfasserin |4 aut | |
| 245 | 1 | 2 | |a A novel 3D coordination polymer constructed by dual-ligand for highly sensitive detection of purine metabolite uric acid |
| 264 | 1 | |c 2021 | |
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| 500 | |a Date Revised 27.07.2021 | ||
| 500 | |a published: Print-Electronic | ||
| 500 | |a Citation Status MEDLINE | ||
| 520 | |a Copyright © 2021. Published by Elsevier B.V. | ||
| 520 | |a Uric acid (UA), as the final product of purine metabolism, exists in urine and serum, which plays an important role in human metabolism, immunity and other functions. The sensitive, efficient, and rapid detection of UA has far-reaching significance in clinical diagnosis and disease prevention. Herein, a novel coordination polymer constructed by dual-ligand was successfully prepared, which exhibited excellent thermal and water stability. The polymer was interlaced by coordination bonds and hydrogen bonds to form an infinitely extended three-dimensional framework, which showed a rare and novel topological structure. The complex selectively recognized UA through significant fluorescence quenching response in the presence of various interferences. The excellent detection sensitivity (the limited detection of 1.2 μM), outstanding anti-interference ability and remarkable recyclability marked the complex to be a promising sensor material towards UA. In addition, the detection mechanism of UA by the complex was investigated in detail by combining density functional theory (DFT) and a variety of other analytical methods | ||
| 650 | 4 | |a Journal Article | |
| 650 | 4 | |a Coordination polymer | |
| 650 | 4 | |a Fluorescent sensor | |
| 650 | 4 | |a Photoinduced electron transfer (PET) | |
| 650 | 4 | |a Purine metabolite | |
| 650 | 4 | |a Uric acid (UA) | |
| 650 | 7 | |a Ligands |2 NLM | |
| 650 | 7 | |a Polymers |2 NLM | |
| 650 | 7 | |a Uric Acid |2 NLM | |
| 650 | 7 | |a 268B43MJ25 |2 NLM | |
| 700 | 1 | |a Yang, Qi-Shan |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Jia |e verfasserin |4 aut | |
| 700 | 1 | |a Fu, Dong-Lei |e verfasserin |4 aut | |
| 700 | 1 | |a Jiang, Dao-Kuan |e verfasserin |4 aut | |
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