Polar meron lattice in strained oxide ferroelectrics

A topological meron features a non-coplanar structure, whose order parameters in the core region are perpendicular to those near the perimeter. A meron is half of a skyrmion, and both have potential applications for information carrying and storage. Although merons and skyrmions in ferromagnetic materials can be readily obtained via inter-spin interactions, their behaviour and even existence in ferroelectric materials are still elusive. Here we observe using electron microscopy not only the atomic morphology of merons with a topological charge of 1/2, but also a periodic meron lattice in ultrathin PbTiO3 films under tensile epitaxial strain on a SmScO3 substrate. Phase-field simulations rationalize the formation of merons for which an epitaxial strain, as a single alterable parameter, plays a critical role in the coupling of lattice and charge. This study suggests that by engineering strain at the nanoscale it should be possible to fabricate topological polar textures, which in turn could facilitate the development of nanoscale ferroelectric devices.

Medienart:

E-Artikel

Erscheinungsjahr:

2020

Erschienen:

2020

Enthalten in:

Zur Gesamtaufnahme - volume:19

Enthalten in:

Nature materials - 19(2020), 8 vom: 01. Aug., Seite 881-886

Sprache:

Englisch

Beteiligte Personen:

Wang, Y J [VerfasserIn]
Feng, Y P [VerfasserIn]
Zhu, Y L [VerfasserIn]
Tang, Y L [VerfasserIn]
Yang, L X [VerfasserIn]
Zou, M J [VerfasserIn]
Geng, W R [VerfasserIn]
Han, M J [VerfasserIn]
Guo, X W [VerfasserIn]
Wu, B [VerfasserIn]
Ma, X L [VerfasserIn]

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Date Revised 19.01.2021

published: Print-Electronic

Citation Status PubMed-not-MEDLINE

doi:

10.1038/s41563-020-0694-8

funding:

Förderinstitution / Projekttitel:

PPN (Katalog-ID):

NLM310635934