Determination and Source Apportionment of Aromatic Acids in PM2.5 from the Northern Suburb of Nanjing in Winter
Atmospheric particulate samples of PM2.5 were collected from the northern suburb of Nanjing in December, 2014, and a LC-MS method was optimized for the determination of aromatic acids in PM2.5; The concentrations of major water-soluble ions, organic carbon and elemental carbon were also determined. The quantification results showed that the average total concentration of five aromatic acids we have determined was (50.01±16.05) ng·m-3, and the average concentrations of terephthalic acid, phthalic acid, trimellitic acid, 4-methylphthalic acid and iso-phthalic acid were (34.54±12.79)、(8.14±3.34)、(2.27±1.39)、(1.68±0.77) and (1.08±0.43) ng·m-3, respectively. The different source apportionments of atmospheric particulate were analyzed by principal component analysis/absolute principal component scores (PCA/APCS) receptor model. The results of source apportionment showed that the main sources of Phthalic acid, Trimellitic acid and 4-methylphthalic acid were mainly secondary transformation, and primary emissions such as vehicle exhaust contributed less to Trimellitic acid; Secondary transformation and biomass burning made the most significant contributions to iso-Phthalic acid and vehicle exhaust contributed less; The sources of Terephthalic acid were primary emissions such as biomass burning and vehicle exhaust.
Medienart: |
E-Artikel |
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Erscheinungsjahr: |
2016 |
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Erschienen: |
2016 |
Enthalten in: |
Zur Gesamtaufnahme - volume:37 |
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Enthalten in: |
Huan jing ke xue= Huanjing kexue - 37(2016), 7 vom: 08. Juli, Seite 2436-2442 |
Sprache: |
Chinesisch |
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Beteiligte Personen: |
Zhang, Ya-Fei [VerfasserIn] |
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Links: |
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Themen: |
Benzene polycarboxylic acids |
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Anmerkungen: |
Date Completed 16.10.2018 Date Revised 16.10.2018 published: Print Citation Status PubMed-not-MEDLINE |
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doi: |
10.13227/j.hjkx.2016.07.004 |
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funding: |
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Förderinstitution / Projekttitel: |
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PPN (Katalog-ID): |
NLM286075288 |
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520 | |a Atmospheric particulate samples of PM2.5 were collected from the northern suburb of Nanjing in December, 2014, and a LC-MS method was optimized for the determination of aromatic acids in PM2.5; The concentrations of major water-soluble ions, organic carbon and elemental carbon were also determined. The quantification results showed that the average total concentration of five aromatic acids we have determined was (50.01±16.05) ng·m-3, and the average concentrations of terephthalic acid, phthalic acid, trimellitic acid, 4-methylphthalic acid and iso-phthalic acid were (34.54±12.79)、(8.14±3.34)、(2.27±1.39)、(1.68±0.77) and (1.08±0.43) ng·m-3, respectively. The different source apportionments of atmospheric particulate were analyzed by principal component analysis/absolute principal component scores (PCA/APCS) receptor model. The results of source apportionment showed that the main sources of Phthalic acid, Trimellitic acid and 4-methylphthalic acid were mainly secondary transformation, and primary emissions such as vehicle exhaust contributed less to Trimellitic acid; Secondary transformation and biomass burning made the most significant contributions to iso-Phthalic acid and vehicle exhaust contributed less; The sources of Terephthalic acid were primary emissions such as biomass burning and vehicle exhaust | ||
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